Nonclassical Radiation from Thermal Cavities in the Ultrastrong Coupling Regime

Thermal or chaotic light sources emit radiation characterized by a slightly enhanced probability of emitting photons in bunches, described by a zero-delay second-order correlation function $g^{(2)}(0) = 2$. Here we explore photon-coincidence counting statistics of thermal cavities in the ultrastrong coupling regime, where the atom-cavity coupling rate becomes comparable to the cavity resonance frequency. We find that, depending on the system temperature and coupling rate, thermal photons escaping the cavity can display very different statistical behaviors, characterised by second-order correlation functions approaching zero or greatly exceeding two.Comment: results on frequency resolved photon correlations added, to appear in Phys. Rev. Let

Photon correlations from ultra-strong optical nonlinearities

We study the full field and frequency filtered output photon statistics of a resonator in thermal equilibrium with a bath and containing an arbitrarily large quartic nonlinearity. According to the general theory of photodetection, we derive general input-output relations valid for the ultra-anharmonic regime, where the nonlinearity becomes comparable to the energy of the resonator, and show how the emission properties are modified as compared to the generally assumed simple anharmonic regime. We analyse the impact of the nonlinearity on the full statistics of the emission and its spectral properties. In particular we derive a semi-analytical expression for the frequency resolved two-photon correlations or two-photon spectrum of the system in terms of the master equation coefficients and density matrix. This provides a very clear insight into the level structure and emission possibilities of the system.Comment: 10 pages, 7 figure

All Optical Switch of Vacuum Rabi Oscillations: The Ultrafast Quantum Eraser

We study the all-optical time-control of the strong coupling between a single cascade three-level quantum emitter and a microcavity. We find that only specific arrival-times of the control pulses succeed in switching-off the Rabi oscillations. Depending on the arrival times of control pulses, a variety of exotic non-adiabatic cavity quantum electrodynamics effects can be observed. We show that only control pulses with specific arrival times are able to suddenly switch-off and -on first-order coherence of cavity photons, without affecting their strong coupling population dynamics. Such behavior may be understood as a manifestation of quantum complementarity

Photodetection probability in quantum systems with arbitrarily strong light-matter interaction

Cavity-QED systems have recently reached a regime where the light-matter interaction strength amounts to a non-negligible fraction of the resonance frequencies of the bare subsystems. In this regime, it is known that the usual normal-order correlation functions for the cavity-photon operators fail to describe both the rate and the statistics of emitted photons. Following Glauber's original approach, we derive a simple and general quantum theory of photodetection, valid for arbitrary light-matter interaction strengths. Our derivation uses Fermi's golden rule, together with an expansion of system operators in the eigenbasis of the interacting light-matter system, to arrive at the correct photodetection probabilities. We consider both narrow- and wide-band photodetectors. Our description is also valid for point-like detectors placed inside the optical cavity. As an application, we propose a gedanken experiment confirming the virtual nature of the bare excitations that enrich the ground state of the quantum Rabi model.Comment: 9 pages, 1 figur

Non-perturbative Dynamical Casimir Effect in Optomechanical Systems: Vacuum Casimir-Rabi Splittings

We study the dynamical Casimir effect using a fully quantum-mechanical description of both the cavity field and the oscillating mirror. We do not linearize the dynamics, nor do we adopt any parametric or perturbative approximation. By numerically diagonalizing the full optomechanical Hamiltonian, we show that the resonant generation of photons from the vacuum is determined by a ladder of mirror-field {\em vacuum Rabi splittings}. We find that vacuum emission can originate from the free evolution of an initial pure mechanical excited state, in analogy with the spontaneous emission from excited atoms. By considering a coherent drive of the mirror, using a master-equation approach to take losses into account, we are able to study the dynamical Casimir effect for optomechanical coupling strengths ranging from weak to ultrastrong. We find that a resonant production of photons out of the vacuum can be observed even for mechanical frequencies lower than the cavity-mode frequency. Since high mechanical frequencies, which are hard to achieve experimentally, were thought to be imperative for realizing the dynamical Casimir effect, this result removes one of the major obstacles for the observation of this long-sought effect. We also find that the dynamical Casimir effect can create entanglement between the oscillating mirror and the radiation produced by its motion in the vacuum field, and that vacuum Casimir-Rabi oscillations can occur.Comment: 30 pages, 8 figure

Revealing higher-order light and matter energy exchanges using quantum trajectories in ultrastrong coupling

The dynamics of open quantum systems is often modeled using master equations, which describe the expected outcome of an experiment (i.e., the average over many realizations of the same dynamics). Quantum trajectories, instead, model the outcome of ideal single experiments - the "clicks"of a perfect detector due to, e.g., spontaneous emission. The correct description of quantum jumps, which are related to random events characterizing a sudden change in the wave function of an open quantum system, is pivotal to the definition of quantum trajectories. In this article, we extend the formalism of quantum trajectories to open quantum systems with ultrastrong coupling (USC) between light and matter by properly defining jump operators in this regime. In such systems, exotic higher-order quantum-state and energy transfer can take place without conserving the total number of excitations in the system. The emitted field of such USC systems bears signatures of these higher-order processes, and significantly differs from similar processes at lower coupling strengths. Notably, the emission statistics must be taken at a single quantum trajectory level, since the signatures of these processes are washed out by the "averaging"of a master equation. We analyze the impact of the chosen unraveling (i.e., how one collects the output field of the system) for the quantum trajectories and show that these effects of the higher-order USC processes can be revealed in experiments by constructing histograms of detected quantum jumps. We illustrate these ideas by analyzing the excitation of two atoms by a single photon [Garziano, Phys. Rev. Lett. 117, 043601 (2016)0031-900710.1103/PhysRevLett.117.043601]. For example, quantum trajectories reveal that keeping track of the quantum jumps from the atoms allows one to reconstruct both the oscillations between one photon and two atoms as well as emerging Rabi oscillations between the two atoms

Dissipation and Thermal Noise in Hybrid Quantum Systems in the Ultrastrong Coupling Regime

The interaction among the components of a hybrid quantum system is often neglected when considering the coupling of these components to an environment. However, if the interaction strength is large, this approximation leads to unphysical predictions, as has been shown for cavity-QED and optomechanical systems in the ultrastrong-coupling regime. To deal with these cases, master equations with dissipators retaining the interaction between these components have been derived for the quantum Rabi model and for the standard optomechanical Hamiltonian. In this article, we go beyond these previous derivations and present a general master equation approach for arbitrary hybrid quantum systems interacting with thermal reservoirs. Specifically, our approach can be applied to describe the dynamics of open hybrid systems with harmonic, quasi-harmonic, and anharmonic transitions. We apply our approach to study the influence of temperature on multiphoton vacuum Rabi oscillations in circuit QED. We also analyze the influence of temperature on the conversion of mechanical energy into photon pairs in an optomechanical system, which has been recently described at zero temperature. We compare our results with previous approaches, finding that these sometimes overestimate decoherence rates and understimate excited-state populations